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  4. Recovery of submicron particles using high-throughput dielectrophoretically switchable filtration
 
Zitierlink DOI
10.26092/elib/2453
Verlagslink DOI
10.1016/j.seppur.2014.06.028

Recovery of submicron particles using high-throughput dielectrophoretically switchable filtration

Veröffentlichungsdatum
2014-06-25
Autoren
Pesch, Georg R.  
Du, Fei  
Schwientek, Udo  
Gehrmeyer, Caspar  
Maurer, Alexander  
Thöming, Jorg  
Baune, Michael  
Zusammenfassung
Conventional methods for separation of submicron particles, e.g., filtration or centrifugation, suffer from severe problems, such as loss of particles during resuspension and high energy demands due to fouling of separating membranes. Here we present the novel concept of dielectrophoretically switchable filtration using pore sizes that are two to three orders of magnitude larger than the particles. We used layer-by-layer (LbL) assembled nanocapsules of 340 nm diameter that were to be separated and recovered from polyelectrolyte solution. The filter being an insulating porous structure is placed in between two electrodes generating an electric field which is bend at the solid–liquid interface and is thus highly inhomogeneous. Dielectrophoresis (DEP) is used as a driving force to trap particles in the filter. The filtration is based on electric effects and could thus be easily turned off by switching off the electric field allowing safe and easy resuspension of the trapped nanocapsules. A parametric study has been conducted to investigate the influence of voltage, pore size, flux and membrane thickness on the separation efficiency. Maximum separation and recovery efficiencies in a semi-continuous run reached almost 65% when working with a specific flow rate of 4.12 mL s−1 m−2, a voltage of 200 V, frequency of 210 kHz and a filter with thickness of 1.5 mm and pore sizes in the range of 20–60 μm. The results demonstrate that electrically switchable retardation of nanoparticles is possible even in large flow systems. This finding paves the way for preparative DEP chromatography of nanoparticles. Its ease makes this switchable filtration attractive for nanoparticle separation and purification in general.
Schlagwörter
Microparticles

; 

Nanoparticles

; 

Separation efficiency

; 

Insulator-based dielectrophoresis

; 

Membrane fouling

; 

Mimenima
Verlag
Elsevier
Institution
Universität Bremen  
Fachbereich
Zentrale Wissenschaftliche Einrichtungen und Kooperationen  
Institute
Zentrum für Umweltforschung und nachhaltige Technologien (UFT)  
Dokumenttyp
Artikel/Aufsatz
Zeitschrift/Sammelwerk
Separation and Purification Technology  
Band
132
Startseite
728
Endseite
735
Seitenzahl
8
Zweitveröffentlichung
Ja
Dokumentversion
Postprint
Lizenz
https://creativecommons.org/licenses/by-nc-nd/4.0/
Sprache
Englisch
Dateien
Lade...
Vorschaubild
Name

G.R. Pesch, F. Du. U, Schwientek, C. Gehrmeyer, A. Maurer, J. Thöming, M. Baune, Recovery of submicron particles using high-throughput_2014_accepted version.pdf

Size

1.17 MB

Format

Adobe PDF

Checksum

(MD5):a3053fe3f93088bfed86a90135bfbe58

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